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Search for "bioinspired conjugates" in Full Text gives 1 result(s) in Beilstein Journal of Nanotechnology.

Self-organizing bioinspired oligothiophene–oligopeptide hybrids

Alexey K. Shaytan,
Eva-Kathrin Schillinger,
Elena Mena-Osteritz,
Sylvia Schmid,
Pavel G. Khalatur,
Peter Bäuerle and
Alexei R. Khokhlov

Beilstein J. Nanotechnol. 2011, 2, 525–544, doi:10.3762/bjnano.2.57

effort to reveal the structure of the fibrils at the nanoscale. Based on the combined theoretical and experimental analysis, the most likely models of fibril formation and aggregation are suggested. Keywords: amyloid-like fibrils; bioinspired conjugates; molecular dynamics simulations; oligopeptides

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Figure 1: Various morphological organization examples of fibrillar aggregates that can be formed by polymer b...

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Scheme 1: Synthesis of quaterthiophene-β-sheet-peptide hybrid 1 [22]; (i) Hg(II)OAc₂, CHCl₃, 0 °C → r.t., 14 h; I₂...

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Scheme 2: Synthesis of quaterthiophene-β-sheet-peptide hybrid 6 [23]; (i) POCl₃, DMF, dichloroethane, reflux, 3 h...

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Figure 2: The A–B–A-type hybrid 1 in the deprotected, but still kinked, form 1'.

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Figure 3: AFM height images of hybrid 1' on mica from a 1:1 DCM/MeOH solution; a) left: Network of fibers aft...

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Figure 4: AFM images of the switched PEO–peptide–quaterthiophene–peptide–PEO compound 1 [22].

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Figure 5: A–B system 6' in deprotected, but still kinked, form.

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Figure 6: AFM height images of 6' on mica from a 1:1 DCM/MeOH solution. a) left: Image of fibers obtained aft...

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Figure 7: AFM height and amplitude images of fully switched PEO–peptide–quaterthiophene 6 on mica [23]. a) left: ...

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Figure 8: Calculated minimum energy conformation of oligothiophene–oligopeptide hybrid 1' in the three Cartes...

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Figure 9: a) Schematic representation of hybrid 1. Black coils: PEO chains, green arrow: Peptide strand; yell...

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Figure 10: Model for the self-assembly of hybrid 6', based on the theoretically calculated conformation of 6' ...

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Figure 11: Theoretical analysis workflow (see text).

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Figure 12: Constructed periodic crystalline cells for (a) antiparallel and (b) parallel arrangement of peptide...

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Figure 13: Possible options for the arrangement of β-sheets in a cross-β motif. Two identical sheets can be cl...

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Figure 14: Schematic representations of constructed double-layer periodic arrangements from the hybrid molecul...

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Figure 15: Snapshots of four different types of fibrils at the initial conformation (a1, b1, c1, d1) and after...

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Review

Published 05 Sep 2011

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